Effective second-order susceptibility in photonic crystals mode of centrosymmetric materials

Second harmonic generation from the ‘centrosymmetric’ crystals

Second harmonic generation (SHG) is a well known non-linear optical phenomena which can be observed only in non-centrosymmetric crystals due to non-zero hyperpolarizability. In the current work we observed SHG from a Zn(II) complex which was originally thought to have crystallized in the centrosymmetric space group C2/c. This has been attributed to the unequal antiparallel packing of the metal ...

Active Materials in Photonic Crystals

I analyze new phenomena arising from embedding active materials inside of photonic crystal structures. These structures strongly modify the photonic local density of states (LDOS), leading to quantitative and qualitative changes in the behavior of active materials. First, I show that the emission spectrum of pointlike sources inside an “omniguide” is strongly modified by features resembling one...

Second-order polarization-mode dispersion in photonic crystal fibers

Redetermination of second-order susceptibility of zinc oxide single crystals.

We measured the second-harmonic signal generated by high-quality zinc oxide single crystals. Comparing this signal with that generated by single-crystal quartz, used as a standard, we found that the components of the second-order susceptibility tensor differ somewhat from the values reported earlier. Measurements of two zinc oxide single crystals with different orientations yield similar results.

Controlling the effective second-order susceptibility in random quadratic media.

We study systematically the effect of spatial disorder of ferroelectric domains in nonlinear media on the polarization properties of optical frequency conversion. Experimentally, different statistics of domain sizes are created using electric field poling at room temperature. We analyze the evolution of polarization properties of the second- and third-harmonic signals for each created statistic...